Well, not sure if this is terminal yet but... received the brackets and went straight to work. Added some little rubber O-rings to increase the pressure on the chip as mentioned in another guide (not excessively tight), and installed the card again without the shroud and a 92mm fan. Temps on GPU2 were going upto 97C in furmark. Obviously this wasn't working as well as I wanted, and I had used the old paste again, but the card ran fine.
Decided to just try with the standard pressure so removed the rubber ring, cleaned the GPU's and intermidary chip, and used new paste etc (spread evenly). Went into windows, checked idle temps, and straight away I can see they are much reduced at idle. 35-38C GPU1 and 45-47C GPU2. So, of course thought I'd test it as per usual for temps. Ran furmark multi-GPU, as I have done for all the other checks to try and get a stable temp for short periods (pretty much emulates Crysis temps), and easier to terminate etc. Temps were much improved with GPU2 only going up about 64C. That's about a 30C decrease so far. Ok temps were still slowly going up, but not as rapidly as before, and the fan wasn't that noisy for a change
Then I hit 65C. Furmark froze, a few coloured artifacts but the fan and everything still going in the background. Waited a short time until the HDD wasn't chugging then turned off the PC. Waited a moment or so, then booted up again, and it said a device not installed or something, then I looked at the MSI AB, and GPU, and it was only showing my 4870X2 as having one core available and crossfire disabled. OK, I admit it, a slight worry did creep in at that point. So ran furmark anyway.. all seemed ok bizarrely. I rebooted the PC anyway, and on the next go after a short moment, the screen went black. HDD still going in the background etc though.
So to cut it short, I have attempted several times now to reinstall the Blocks and new paste but still getting black screen. Sometimes it happens when I get into windows and the gfx driver has loaded (it actually is searching for it and say's it is installing (a generic driver?)... which makes me concerned, and other times it freezes at the windows bootup screen.
Annoyingly I can't remove Catalyst when in safe mode, and not quick enough to try and uninstall yet lol.
Obviously I'm concerned I'm doing something wrong with the bracket installation. Do the screw springs need some spring left in them, or am I meant to do the block right up? (I did it right up so each of the black pads on the X-bracket are contacting the pcb.)
It's either that, or it simply had an unfortunate crash and corrupted something (likely the drivers)
Obviously hoping I haven't damaged anything!