That's a tough question to answer. I was originally lead to believe that timings were much more important that FSB now that the memory controler is on the CPU, but i've certainly found that FSB still makes a hugh difference. I was running my ram at something like 186 on a 133 divider to get the most of my opty 144, but I decided to just see what would happen if I went back up to 166. In all fairness my timings were not great at 186 just 2-3-3-6 (i wasn't bothering to fiddle) and they remained the same when I went back to 166, so this is only a differentiation between FSB speeds. But anyway, going from 186 to 240 FSB took 3 mins of my superpi32m time. I was expecting it to be better, but that was a bigger jump than going from 2.4 to 2.6ghz.
I think what you really want is ram that will get somwhere in the 220-250 region but keep decent timings in the region of 2-3-2-6 to 2.5-3-3-6, then go with a small divider to go that last mile. The PC4000 that gets 3-4-4-8 i'd rule out. Instead go for somthing that can be pushed a bit in terms of FSB (not necessarily to 270+, but at least 220-230) but does so with good timings. I highly recommend the XMS3500 but as you're using a DFI i'd plump for low latency PC3200. OZC platinum is pretty good and does well on those boards from what i've read. You should get similar results to me.