I don't really know about how far you could overclocked using that mainboard, although from the memory i'm guessing you won't have much headroom if any. You'd probably have more success with some 667 or even better, some 800.
And for a cooler, I've heard lots of good things about (and will be getting) the Arctic Cooling Freezer 7 Pro. Outperforms coolers of twice the price and it's under 18 quid inc. Vat at OcUK. Link here. Comes with thermal paste pre-applied as well.
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