TFC Shrouds and shrouds in general - Always provide a good performance benefit and reduce noise at the same time. Highly recommended in all radiator setups particularly for higher speed fans unless the space does not make them an option. You can see as much as 10-16% gains on higher speed 38mm fans and 6% gains with slow speed fans. Generally the higher the fan speed and the larger the fan hub, the more gain you will see with shrouds. Optimal depth appears to be somewhere around 30mm +-, this is likely to depend on hub diameter and RPM to some extent.
Push Vs Pull - This depends on fan speed/power. The high speed fans at 2000RPM with a 38mm fan thickness provided the best performance in a push condition. The slow speed fans with 1350RPM with a 25mm fan thickness provided the best performance in a pull condition. I would estimate that performance line is likely to cross in the 1500-1700RPM range where they are equal. So.... slow speed = pull, high speed = push, medium speed = it doesn't really matter.
2 fans Push/Pull vs others - It was very clear that when using two fans per radiator section, that the radiator intself acts as a flow spreader and provided great benefit to straightening out the air for the second fan in a push/pull configuration. Just like doubling up with a pump, there is a pressure benefit to doubling up on fans and this translates to about a 20-30% performance gain. The added fan pressure simply means and added gain in air flow and corresponding performance. None of the experimental pull/pull or push/push configurations provided any noteworthy benefit as it seams the air is simply too disturbed from the first fan to allow the second to perform properly when air is moving. I would always recommend a push/pull configuration for two fans and add a shroud to both sides if space allows.