At a guess I would say SLi but I have never seen them compared directly. As for raw power, two X1900 series cards in Crossfire would be faster than any nVidia SLi setup.
It's all a gimmick anyway unless you're benching or have a huge monitor - ie 30".
So if your super rich (got money to burn) go for crossfire. If not SLi, it's so much more supported, but don't feel you need it, a 7900GT will do anything pretty much.
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