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9600GT. But it's not worth it for one game IMO.

I want to play Mirror's Edge and Batman: Dark Asylum, so that's two already.
I'm sure nVidia will push it onto more top games as well.
So anyways, thanks for that - 9600GT it is then, if I can get one dirt cheap.
Are you planning on using the card with your 8800GT?

Yes, but Arkham Asylum is the only game that shows a tangible benefit from having a dedicated card. And even that's tenuous. By all means, buy a card for PhysX if you want, but I can't really recommend it.
Any reasonably decent DX10 card should do - 9600GT, 8800GT, 8800GTS etc.

How would my 8600GTS do? Or should I rephrase that as, is it worth getting anything faster?
I really wouldn't bother getting a card now, Nvidia have a clear intention of not allowing Physx on a ATi system, theres a hack now, but with every new game they can force a new version of Ageia to be needed, and a new gfx driver to support it and a new game to smeg around with all to reblock it. Whatever hack thats there now, will most likely not work in the future if Nvidia set their minds too it.
If you're sticking with Nvidia, by all means do so, but I wouldn't get a new card hoping Nvidia don't make the "hack" to make it work with ATi cards useless in future drivers/ageia drivers/games.