what is your NB temp? like with the CPU, under most normal cooling methods the temps kick up well before the volts by themselves become dangerous.
i need 1.55V NB to hit around 450 FSB with my P5K-Dlx, and that 680i is running at 1.4V atm. Not sure how voltage dependant the FSB is, but some mobos can need quite a lot to hit decent speeds.
Another test, drop the CPU multi a notch and re-test, if you are still getting probs then its the NB not the CPU core that's causing probs, it sure as hell wont be the Mem if you are running unlinked. If that is the case, push the vNB up a notch and try and find the max FSB at that setting (watching the NB temps with whatever monitor you use), which will give you a range up to which you can push to explore the overclocking potential of your CPU without getting errors that COULD be CPU or NB based.
Remember overclocking 101; find the INDEPENDANT limits of each component in your system before trying to find the best stable mix of those maximums.
eg:
Step 1: set mem to max safe volts for your DIMMS, with the slackest timings you are prepared (5-5-5-18 is about the furthest i go), up the mem multi, drop the CPU multi, and raise the FSB notch by notch untill you find the max stable mem speed (with raised multi this should not be FSB limited), or for RD600/650i/680i unlink the mem and find the max stable async speed.
Step 2: set mem to 1:1 with loosest timings (or async if poss), raise NB to max safe volts, drop CPU multi, and attempt to find max stable FSB for the board, or the max stable mem speed if 1:1 (may still be CPU limited, as some cpus have an "FSB wall" past which further increases are unstable).
Step 3: set mem to 1:1 with loosest timings (or async), vNB to max safe, vCore to max safe, CPU multi to max and slowly increase FSB untill you either hit your FSB limit, or you get instabilities or unsafe load temps.
Step 4: mix & match, try to get the best mix of CPU speed and mem speed using the avaliable combinations of memory and CPU dividers. Optimum is of course having max mem @ 1:1, with high FSBs/low CPU multi, but you may have to drop the FSB, and increase the CPU multi/Mem divider to hit the optimum mix. Having Async mem can be a real benefit if you want to max your mem, or have poor OCing mem, as you can optimise the CPU independant of the Mem.
Step 5: Long stability test of completed combined OC
Voila..... beautiful stable, maxed out system!