The above will move what I would call the personal documents area over to another folder/drive. You can also change the default folder for profiles by modifying this registry key
Any new users created would then by default have their profile created in the folder you set in ProfileList.
Be warned though, I'd leave the admini user still on the C: drive as if the other drive/folder cannot be accessed you won't even be able to logon as admin.
EDIT: You'll need to also copy over the All Users and Default User folders and any existing users will need their registry altered to reflect the new location. The keys you'll need to change are:
Last question, what if a an application (say a game or something) has hardcoded the path to the default (c:\docs and sets or w/e it is!). Will windows redirect it? or will it try place its settings/files into the old location?
All depends where the game is getting that location from, if it's in the registry hard pathed then find it and change it, if it's preceded by %USERPROFILE% then the game will use the new location.
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