Given the CPU is over 3years old, i'd also delid it.. I'm sure you'll see a much better improvement over what you have now.
If you do go that route would be interesting to see temp difference between a direct die mount or LM on die, Kryonaught on lid mount.
I'm running direct die on my 4770K o/c to 4.5. Don't have temps before (as Photobucket deleted all my photos after it went to that silly paid service) but my temps idle mid 30s and load at around 60c.. and the 4770K is a toasty chip