drop your package power to 100 and leave EDC @ 140 and TDC @ 90 you should see significant drop in temps
default motherbaord package power is 140W for 5800X the default for the chip is 105w.
with all those settings on auto or not altered, you are using the maximum thermal and electrical current specification for the chip. if you want temps to be inline with the default spec for 5800X then drop the package power down.
I am on LF2 360mm and it can manage the 140W output just fine. mid 70c after a couple of hours of aida64 with P12 fans kicking in at 70% rpm.
at 120w (which is my current profile) the 2hr torture test yield mid 60c fans run at 60%RPM.
my fan profile is 40% upto 50c 60% upto 70c then 70% for anyting beyond with step change no gradual fan speed change.
I followed your recommendations earlier, been using my PC all evening and it's made a 'massive' difference, I still seem to have all of the performance yet my temperatures and thus fan speeds and therefore noise have dropped hugely, running repeat multithreaded runs over Cinebench now it sits at 72c, it's like a different system. Because I still have all of the performance because it's not throttling itself due to hitting 90c anymore, I do think once I put the AIO on ...well later today at this point (didn't realise it was 01:20 tbh) it will open up headroom to run faster, maybe I could see 5ghz boosts on 1 or 2 cores etc, I wonder, what I do know is I am happy right now with it, I've still ordered the cooler of course but right now I see that as an opportunity to tune this up a bit now

Edit: Actually when I said 'all' of the performance, there is a very slight difference, in the very short time before it was dialling back the clock speed after hitting 90c (this was something like 30 seconds), it was boosting higher on all cores than it does now infact but then with 140w Package Power I guess it would, but it's ability to sustain that was so short lived it didn't amount to much and was a lot less pleasant to use because uber turbo fan speeds were being maintained while it sat at 90c and the boost difference was only about 100mhz all core, I can probably get that back with the AIO and some tweaking tbh, at least that I would guess.
This is the key to getting the most out of these I think now, not necessarily throwing more cooling at it, but understanding how to tune it with what you do have, obviously I am happy to spend money on more so I guess I will benefit from that ...I'll find out later anyway.
The exact settings I have in use now are,
CPU TDC set to 90A
CPU EDC set to 140A
CPU PPT set to 105W
Curve Optimizer
Negative
20
@pc-guy and @humbug thanks so much for your advice so far, it's really made a nice difference.
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