My settings for 3.6 (my chip is a 1.3 VID)...
External Clock - 400
Multiplier - 9x
DRAM Speed - 1:1:25 (DDR2-1000)
PCI-E - 100
CPU - 1.52v (1.42 or so under load)
DDR2 - 2.0v
CPU VTT - 1.23v
MCH - 1.29v
ICH - 1.05v
ICHIO - 1.5v
DDR2 REF - 0%
CPU GTL 0+2 - 67%
CPU GTL 1+3 - 67%
Limit CPUID MaxVal - Disabled
C1E - Auto
Execute Disable Bit - Enabled
Virtualisation - Disabled
EIST - Auto
RAM - By SPD
...you will need to watch the PWM temps. My board is bolt modded and I have a 60mm fan hovering above the PWM area keeping them cool. You may well need the bolt mod if it's not already done...
http://www.xtremesystems.org/forums/showpost.php?p=2330347&postcount=751
I also have 2x 40mm fans on the Northbridge, as it can get pretty toasty too.
Bear in mind that the above setting was when I was running 4gb RAM. I am still at 3.6 with 8gb, but have to run the memory on a different divider so that it runs at 800mhz. Any more was too much for the board to cope with.
EDIT - for what it's worth I found that anything above 1.3 for the MCH would cause instabilities. For some reason my board prefered the MCH to be kept fairly low.