A radiators(as name implies) are designed to radiate energy (hot or cold) energy and not to store energy. The bigger the radiator the more tube area and surface area it has and the more heat it can radiate.
More air movement through radiator means more heat can be radiated.
CFM
H100i has 2x 77cfm fans so a total of 154cfm maximum flow
Kraken is 2x 98.3cfm fans so total of 197.6 cfm max.
Static pressure
H100i is 4mm H2O
X60 has 2.2 mm-H2O
Less static pressure but still respectable amount.
I can't find any specs of radiator core/fin density or airflow resistance.
I'm guessing the difference between airflow and static pressure will end up with about the same air coming out of respective radiators. If that is the case than the difference ends up being the X60's 35% bigger radiator.
But even if the X60 ends up with 20% less air coming out it will still end up cooling better because radiator is 35% bigger... at least that's my guess
And it's all guessing until both cooler are tested side by side.